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14 декабря, 2021
Fission probabilities have important implications both on the neutron production of the p-nucleus reaction and on the production of nuclear waste. Figure 6.3 compares experimental fission cross-sections for the highly fissile 235U to calculations using the Bertini code with or without
Neutron Momentum (MeV/c) Neutron Momentum (MeV/c) Figure 6.2. Comparison of experimental neutron energy spectra following the reaction p + 7Li with spectra calculated using the Bertini and ISABEL INC codes [90]. Light dots: Bertini; solid line: ISABEL; thick dots: data. |
pre-equilibrium treatment. It is seen that, in this case, the pre-equilibrium treatment does not influence the results very much. This is a consequence of the very high fission probability. For neutron energies below 100 MeV, all INC calculations become unsatisfactory. This reflects a deficiency of the INC codes in reproducing reaction cross-sections below that energy. Figure 6.4 compares experimental fission cross-sections for the poorly fissile 208Pb with calculations using the Bertini and the ISABEL INC codes
Figure 6.3. Comparison of experimental neutron induced fission cross-sections of 235U with calculations based on the Bertini INC with or without pre-equilibrium [90]. Solid line: standard pre-equilibrium MPM calculation [109]. Dashed line: no pre-equilibrium step. Dotted line: hybrid MPM. See Prael [90] for details. |
with or without pre-equilibrium treatment, and for different level densities. Here the interest of the pre-equilibrium treatment is far from obvious. The standard level density is that of Igniatyuk [101] and gives the best results. The Julich level density [84] includes the effects of shells on level densities but not the washing out of these effects with temperature. It clearly underestimates the level density. In any case, as stated earlier, it seems clear that progress has to be made in the fission treatment.