ACCELERATOR DRIVEN SUBCRITICAL REACTORS

Introduction

Although, at the beginning of nuclear energy deployment, many different reactor systems were proposed and more or less tested, only a few of them became standard in the Western hemisphere: light-water reactors like the PWR (pressurized water reactor) or BWR (boiling water reactor), heavy — water reactors of the CANDU (Canadian deuterium uranium) type and, finally, the sodium cooled fast-neutron reactors (LMR: liquid metal reactor). It was clear from the beginning that breeder reactors like the LMR were necessary for a sustainable development of nuclear power. However, the experience with the LMR is far from conclusive, especially since the universally used sodium coolant seems to lead to too strong safety constraints on the building and operation of the reactors. Further­more, light-water reactors are plagued by the problem of radioactive waste which, to date, has not found a consensual solution. The waste problem added to the fear of catastrophic accidents (Chernobyl syndrome) explains the large societal opposition to nuclear power observed in many countries. To some extent one may think that nuclear energy will come to a dead end. This is an unfortunate situation when the rising concern about the greenhouse effect pleads for a severe reduction in the use of fossil fuels. The development of safer and less polluting means of producing energy from nuclear fission is, thus, of great relevance.

In this context, in recent years, a great deal of interest has been displayed, worldwide, in accelerator driven subcritical nuclear reactors (ADSR or ADS), also called subcritical or hybrid reactors, to produce energy and transmute radioactive wastes in a, possibly, cleaner and safer way than at present. Pioneers in this revival have been Furukawa [1], Bowman [2] and Rubbia [3]. Similar ideas were first proposed more than 50 years ago [6-16]. At that time they were not carried through, not so much because of technical difficulties but for lack of economic incentive. It is true, also, that while building reliable GeV accelerators achieving intensities of several tens of milli — amperes was by no means considered to be a trivial matter, efficient critical reactors were available, and were thus thought to be the simplest and most natural way to harness nuclear fission. It was, however, acknowledged that accelerator driven nuclear devices might offer interesting transmutation possibilities. For example, without a large enough concentration of 235U in natural uranium, the only way to exploit fission energy would have been the use of such subcritical systems.[1]

High-energy accelerators appear to be a promising way to incinerate heavy actinides [17, 18]. It has also been acknowledged that a thorium — based fuel cycle would considerably limit the amount of transuranic wastes produced. The implementation of such a cycle would be made easier with subcritical reactors, due to the improved neutron economy of such systems as compared with classical critical reactors [1-3]. Hybrid reactors appear to be a credible alternative to fast breeder and fusion reactors.

In chapter 2 we examine the general question of world energy needs and possible supplies. In chapter 3 we give an elementary reminder of reactor theory. Chapter 5 is devoted to the description of commonly used reactor simulation codes. In chapter 6 we describe the basic physics of hybrid reactors, including an account of the experimental and computational state of the arts of spallation reactions. In chapter 7 we discuss safety questions specific to ADSRs. In chapter 8 we examine the evolution of hybrid reactor fuel as a function of time. This evolution determines the most impor­tant constraints on the neutronics of hybrid reactors. Chapter 9 describes the main fuel reprocessing techniques, since these condition the possibility of implementing a durable nuclear energy production. Chapter 10 shows how the existence of a spatially confined neutron source influences the size of the reactor. Chapter 11 examines the possible use of hybrid reactors in the nuclear waste issue. Chapter 12 gives some examples of ‘historic’ projects which used either solid or liquid fuels. Chapter 13 discusses the present state of thoughts for the possible development of ADSRs.

In this book we have, deliberately, chosen to place the emphasis on simple, intuitive, treatments of the different aspects of the physics of hybrid reactors, in order to provide the reader with the possibility of gaining physical insight into these systems. However, the reader should be aware that realistic calculations require the use of complex codes, most frequently of the Monte Carlo type. Nevertheless, it is our experience that starting with simple models helps the understanding of the results of the ‘real’ calculations, and provides intuition of the most fruitful ways to improve systems or discover new ones. As far as possible this review is self-contained and does not require a priori knowledge of the field. It elaborates on reviews of the subject previously published in Progress in Particle and Nuclear Physics [4] and in Nuclear Instruments and Methods [5].

In many cases it can be seen that critical reactors could do as well as ADSRs. We hope that this book will give the reader the elements needed to form an opinion on the possible usefulness of ADSRs, as well as to have a good basis for starting working on these systems. More generally, students and practitioners in nuclear reactor technology might find useful the more recent developments presented here.

Acknowledgments

We thank the ISN group, and especially Professor J M Loiseaux, Dr D Heuer, A Nuttin and F Perdu, for contributing to many ideas and much of the material presented here. Professor C Rubbia was the originator of our interest in the subject of hybrid reactors and the main inspiration for our thoughts on the subject. We enjoyed many fruitful interactions with Professors J P Schapira, M Salvatores, M E Brendan and C D Bowmann. Professors D Hilscher, L Tassan-Got, W Mittig, B Lott and S Leray were kind enough to provide us with originals of their figures. Mrs E Huffer was kind enough to read our manuscript carefully and correct the English. The patience and support of Helene Meplan and Marguerite Nifenecker are gratefully acknowledged.