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14 декабря, 2021
Radiation growth of uranium is another form of dimensional instability that occurs under irradiation without the need of any stress in a lower temperature (i. e.,
Figure 7.7 Suitable amount of molybdenum addition can modify the kinetics of alpha-or gamma — phase uranium and remove the thermal cycling growth effect. Taken from Ref. [2]. |
around 300 °C) regime. Since it does not require stress to occur, it is not considered radiation-induced creep. Also, since the volume of the material remains constant during radiation growth, it is not considered as irradiation swelling. Under radiation exposure, a single crystal of alpha-uranium expands in the [010] direction, contracts along the [100] direction, and remains more or less unaltered in the [001] direction. The result of this characteristic expansion/contraction is that the volume remains essentially constant. However, in order for radiation growth to take place, single crystal of uranium is not essential but polycrystalline uranium strong crystallographic texture can also exhibit the effect. Deformation processing and heat treatment is important to minimizing or eliminating the radiation growth effect by suitable texture engineering. Minimization of radiation growth can be achieved by processing the material to produce a fine-grained microstructure with randomly oriented grains. Also, suitable alloying additions to stabilize isotropic phases can help.
The radiation growth coefficient (Gt) is given by Percentage length increase
Percentage atom burnup
There have been a number of studies to understand radiation growth, but it remains elusive. A leading hypothesis of radiation growth by Buckley [ ] is based on differential directional rates of interstitial atoms and vacancies. The interstitials have a tendency to migrate along the [010] direction and to the vacancies in the [100] or [001] directions, leading to basically removal of mass from one side and plating them on the other side. Figure 7.8 shows the irradiation growth effect in a uranium fuel against the fuel burnup.