Experimental and computational evaluation of the response of a SiC neutron monitoring system in a thermal neutron field

Silicon carbide (SiC) is an interesting material for nuclear-reactor power monitor detectors. It has a wide band-gap, small volume and high break down electric field. In addition, SiC is chemically and neutronically inactive. Using SiC power monitors as in-core detectors provides the ability for high counting rate that may help to increase the safety margins of nuclear reactors. To observe the triton response in the SiC p-n diode, a detector with a 1.56 pm LiF converter (with 95% enriched 6LiF) was used. 6Li atoms in the LiF converter may absorb thermal neutrons and generate 2.05 MeV alpha and 2.73 MeV triton particles (6Li(n,3H)a reaction). An 8 pm Al layer was used to minimize damage in the SiC by blocking all alpha particles. However, most tritons have enough energy to pass through this layer and reach the 4.8 pm SiC active layer. The diameter of the LiF converter is 0.508 cm and the SiC diode area is 1.1 mm x 1.1 mm (diode is a square). The active area of the diode is approximately 0.965 mm2. Upon irradiation in the thermal column (TC) facility, one can observe the triton peak in the recorded detector pulse-height spectra and the concomitant triton induced radiation damage on the detector. A schematic of the detector is shown in Figure 8.

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Fig. 8. Schematic of side view of SiC detector. The diameter of the LiF converter is 0.508 cm and the SiC diode active area is 0.965 mm2 (diode is a square). Only the active region of SiC is shown (Blue and Miller, 2008).

The SiC detector package was connected to a pulse processing system consisting of a preamplifier (ORTEK 142 B) and a digital spectrum analyzer (Canberra DSA 2000). An oscilloscope (Hewlett Packard 54601B, 100 MHz) was used to study the shape of the signal from the amplifier. Bias voltage was provided by the DSA to the detector through the preamplifier. A power monitoring program was used to verify the reactor power that was displayed in the control room. In addition, the degradation of the SiC detectors in the TC’s thermal neutron environment was evaluated in terms of dose and dose rate effects. After irradiating the detector at 455 kW, the count rate per kW decreased by a factor of 2 after 11 hr. The I-V characteristics recorded during pre-irradiation and post-irradiation, confirm degradation of the detectors. A theoretical model of the SiC schottky diode detectors was constructed based on MCNP and TRIM computer codes to study the damage induced by tritons for a given diode detector package configuration in the TC’s thermal neutron environment. The predicted count rate was compared with the experimental results that were obtained in the TC irradiation field using a charge sensitive preamplifier. The
experimental results are in agreement with the predicted response to within a factor of three. I-V measurements show some annealing effects occurring at room temperature. Maintaining the detectors at a higher temperature during irradiation may cause more annealing to occur, thus reducing degradation of the detector. Experiments are necessary to test the degradation of the detector at elevated temperatures, to determine if the effects of annealing are sufficiently great so that the detectors may be useful for neutron power monitoring at high count rates.