Irradiation temperature

With respect to the irradiation environment there are four major variables that determine the duration of the transient. The first three are related to each other: irradiation temperature, temperature gradi­ents, and temperature history. The fourth is strongly synergistic with temperature and is the dpa rate, which will be covered in the following section.

Some temperature histories, especially when gradually falling from one temperature to a lower temperature, produce a shorter transient compared to that of either the starting or final temperature, primarily because such histories tend to accelerate the radiation-induced formation of nickel and silicon-rich phases, especially that of the g phase.1’136 Formation of these phases usually precedes swelling.1

Strong gradients in temperature across thin fuel cladding have also been shown to accelerate the onset of swelling, producing more swelling than what iso­thermal irradiation would produce at either the upper or lower cladding temperature.137,138 The exact cause is unknown but it was speculated that the stress gradients associated with strong tempera­ture gradients might be a contributing factor.

For isothermal irradiation the temperature is an important determinant of the transient duration, not only because it directly impacts diffusion and void nucleation, but also because of its influence on phase stability and phase evolution. However, over the wide range of temperatures experienced in fast reactors, temperature has no effect on the posttransient steady-state swelling rate of 300 series stainless steels at ~1% per dpa.

However, it is frequently assumed that at constant dpa rate there is a peak swelling temperature or peak swelling rate as a function of temperature for swelling of austenitic steels. This persistent misperception is a consequence of the historical use of fast reactors. All ofthe early data on swelling was derived from small fast reactor cores such as EBR-II and DFR, which have strongly peaked dpa rate profiles, both axially and radially. Later studies conducted in larger cores such as that of FFTF showed that assuming a temperature — dependent steady-state swelling rate was incorrect. More careful analyses of other data from these smaller cores also support this point of view.